I don't think you could use NLTK from Jython, since it depends on Numpy which isn't ported to the JVM. If you need NLTK or any other native CPython extension, you might consider using some IPC mechanism to communicate between CPython and the JVM. That being said, there is a project to allow calling CPython from Java, called Jepp:
http://jepp.sourceforge.net/
The reverse (calling Java code from CPython) is the goal of JPype and javaclass:
sourceforge.net/projects/jpype/
pypi.python.org/pypi/javaclass/0.1
I've never used any of these project, so I cant't vow for their quality.