What is the proper way to load up a ListBox?

Question

What is the proper way to load a ListBox in C# .NET 2.0 Winforms?

I thought I could just bind it to a DataTable. No such luck.
I though

Answer 1

To bind to a dictionary you have to wrap it in a new BindingSource object.

MyListBox.DataSource = New BindingSource(Dict, Nothing)
MyListBox.DisplayMember = "Value"
MyListBox.ValueMember = "Key"