With a helper tuple class, either your own or—in .NET 4—the standard ones you can do this:
var init = Tuple.Create(0, 0);
var res = m.Items.Aggregate(init, (t,v) => Tuple.Create(t.Item1 + v.Total, t.Item2 + v.Done));
And res.Item1 is the total of the Total column and res.Item2 of the Done column.