Compute Sum of Column in Datatable , Works 100%
lbl_TotaAmt.Text = MyDataTable.Compute("Sum(BalAmt)", "").ToString();
if you want to have any conditions, use it like this
lbl_TotaAmt.Text = MyDataTable.Compute("Sum(BalAmt)", "srno=1 or srno in(1,2)").ToString();